
Between 1968 and 1972, Bob and Rita Marley, Peter Tosh and Bunny Wailer re-cut some old tracks with
JAD Records in
Kingston and London in an attempt to commercialise The Wailers' sound. Bunny later asserted that these songs "should never be released on an album ... they were just demos for record companies to listen to". Also in 1968, Bob and Rita visited
the Bronx to see
Johnny Nash's songwriter
Jimmy Norman. A three-day jam session with Norman and others, including Norman's co-writer Al Pyfrom, resulted in a 24-minute tape of Marley performing several of his own and Norman-Pyfrom's compositions. This tape is, according to Reggae archivist
Roger Steffens, rare in that it was influenced by pop rather than reggae, as part of an effort to break Marley into the American charts. According to an article in
The New York Times, Marley experimented on the tape with different sounds, adopting a
doo-wop style on "Stay With Me" and "the slow love song style of 1960's artists" on "Splish for My Splash". An artist yet to establish himself outside his native Jamaica, Marley lived in Ridgmount Gardens,
Bloomsbury,
London during 1972

In 1972, the Wailers entered into an ill-fated deal with
CBS Records and embarked on a tour with American soul singer
Johnny Nash. Broke, the Wailers became stranded in London. Marley turned up at
Island Records founder and producer
Chris Blackwell's London office, and asked him to advance the cost of a new single. Since
Jimmy Cliff, Island's top reggae star, had recently left the label, Blackwell was primed for a replacement. In Marley, Blackwell recognized the elements needed to snare the rock audience: "I was dealing with rock music, which was really rebel music. I felt that would really be the way to break Jamaican music. But you needed someone who could be that image. When Bob walked in he really was that image.Blackwell told Marley he wanted The Wailers to record a complete album (essentially unheard of at the time). When Marley told him it would take between £3,000 and £4,000, Blackwell trusted him with the greater sum. Despite their "rude boy" reputation, the Wailers returned to Kingston and honored the deal, delivering the album
Catch A Fire.
Primarily recorded on eight-track at Harry J's in Kingston, Catch A Fire marked the first time a reggae band had access to a state-of-the-art studio and were accorded the same care as their rock'n'roll peers. Blackwell desired to create "more of a drifting, hypnotic-type feel than a reggae rhythm",and restructured Marley's mixes and arrangements. Marley travelled to London to supervise Blackwell's overdubbing of the album, which included tempering the mix from the bass-heavy sound of Jamaican music, and omitting two tracks.

The Wailers' first major label album,
Catch a Fire was released worldwide in April 1973, packaged like a rock record with a unique
Zippo lighter lift-top. Initially selling 14,000 units, it didn't make Marley a star, but received a positive critical reception. It was followed later that year by
Burnin', which included the standout songs "
Get Up, Stand Up", and "
I Shot the Sheriff", which appealed to the ear of
Eric Clapton. He recorded a
cover of the track in 1974 which became a huge American hit, raising Marley's international profile. Many Jamaicans were not keen on the new "improved" reggae sound on
Catch A Fire, but the
Trenchtown style of
Burnin' found fans across both reggae and rock audiences.
During this period, Blackwell gifted his Kingston residence and company headquarters at 56 Hope Road (then known as Island House) to Marley. Housing Tuff Gong Studios, the property became not only Marley's office, but also his home.
The Wailers were scheduled to open 17 shows for the number one black act in the States,
Sly and the Family Stone. After 4 shows, the band was fired because they were more popular than the acts they were opening for. The Wailers broke up in 1974 with each of the three main members pursuing solo careers. The reason for the breakup is shrouded in conjecture; some believe that there were disagreements amongst Bunny, Peter, and Bob concerning performances, while others claim that Bunny and Peter simply preferred solo work.
1974–1981

Despite the break-up, Marley continued recording as "Bob Marley & The Wailers". His new
backing band included brothers
Carlton and
Aston "Family Man" Barrett on drums and bass respectively,
Junior Marvin and
Al Anderson on lead guitar,
Tyrone Downie and
Earl "Wya" Lindo on keyboards, and
Alvin "Seeco" Patterson on percussion. The "
I Threes", consisting of
Judy Mowatt,
Marcia Griffiths, and Marley's wife, Rita, provided backing vocals. In 1975, Marley had his international breakthrough with his first hit outside Jamaica, "
No Woman, No Cry", from the
Natty Dread album. This was followed by his breakthrough album in the United States,
Rastaman Vibration (1976), which spent four weeks on the
Billboard Hot 100. On 3 December 1976, two days before "
Smile Jamaica", a free concert organised by the
Jamaican Prime Minister Michael Manley in an attempt to ease tension between two warring political groups, Marley, his wife, and manager Don Taylor were wounded in an assault by unknown gunmen inside Marley's home. Taylor and Marley's wife sustained serious injuries, but later made full recoveries. Bob Marley received minor wounds in the chest and arm. The shooting was thought to have been politically motivated, as many felt the concert was really a support rally for Manley. Nonetheless, the concert proceeded, and an injured Marley performed as scheduled, two days after the attempt. When asked why, Marley responded, "The people who are trying to make this world worse aren’t taking a day off. How can I?" The members of the group
Zap Pow, which had no radical religious or political beliefs, played as Bob Marley's backup band before a festival crowd of 80,000 while members of The Wailers were still missing or in hiding.

Marley left Jamaica at the end of 1976, and after a month-long "recovery and writing" sojourn at the site of Chris Blackwell's
Compass Point Studios in
Nassau, Bahamas, arrived in England, where he spent two years in self-imposed exile. Whilst there he recorded the albums
Exodus and
Kaya.
Exodus stayed on the British album charts for 56 consecutive weeks. It included four UK hit singles: "Exodus", "Waiting in Vain", "Jamming", and "
One Love" (a rendition of
Curtis Mayfield's hit, "
People Get Ready"). During his time in London, he was arrested and received a conviction for
possession of a small quantity of
cannabis. In 1978, Marley returned to Jamaica and performed at another political concert, the
One Love Peace Concert, again in an effort to calm warring parties. Near the end of the performance, by Marley's request, Michael Manley (leader of then-ruling
People's National Party) and his political rival
Edward Seaga (leader of the opposing
Jamaica Labour Party), joined each other on stage and shook hands.
Under the name Bob Marley and the Wailers eleven albums were released, four live albums and seven studio albums. The releases included
Babylon by Bus, a double live album with thirteen tracks, were released in 1978 and received critical acclaim. This album, and specifically the final track "Jamming" with the audience in a frenzy, captured the intensity of Marley's live performances.
Survival, a defiant and politically charged album, was released in 1979. Tracks such as "Zimbabwe", "
Africa Unite", "Wake Up and Live", and "Survival" reflected Marley's support for the struggles of Africans. His appearance at the
Amandla Festival in
Boston in July 1979 showed his strong opposition to South African
apartheid, which he already had shown in his song "
War" in 1976. In early 1980, he was invited to perform at the 17 April celebration of
Zimbabwe's Independence Day.
Uprising (1980) was Bob Marley's final studio album, and is one of his most religious productions; it includes "Redemption Song" and "Forever Loving Jah".
Confrontation, released posthumously in 1983, contained unreleased material recorded during Marley's lifetime, including the hit "
Buffalo Soldier" and new mixes of singles previously only available in Jamaica.